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No, for any regular language $R$, $R'$ is also regular (regular language is closed under complement). Now, suppose if there exists a non-regular language $L$ whose complement $L'$ is regular when we take the complement of $L'$ we get $L'' = L$ which is not regular and is violating the closure property. So, by the proof of contradiction, no such non-regular language can exist whose complement is regular.
0 0 votes
Prove it by contradiction .

let a language L which is Non regular and whose complement L' is regular.

Now as L' is regular and we know Regular languages are closed under complement so (L')' would also be regular.

But we also know (L')' =L so ultimately we proved  L=Regular but as we considered L as non regular so by contradiction the complement of non regular language can't be regular.
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Detailed Video Solution: Complement of a Non-Regular Language is Always Non-regular

Set of Non-Regular languages is Closed under Complementation Operation.

i.e. Complement of a Non-regular language is always a Non-regular language. 

We can prove it by Contradiction.

Let $L$ be any Non-regular language. Now, for contradiction purpose, Assume $\overline{L}$ be Regular.

Now, Since $\overline{L}$ is Regular, so,  $\overline{\overline{L}} $ = $L$ will be Regular, which Contradicts our assumption that $\overline{L} $ is non-regular. 

So, If $L$ is non-regular then $\overline{L}$ is necessarily non-regular.

We can say that $L$ is Regular if and only if $\overline{L} $ is Regular.

MUST Watch: Closure Properties of Non-Regular Languages

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