Set of Non-Regular languages is Closed under Complementation operation, But Not closed under Union or Intersection Operation.
MUST Watch this: Closure Properties of Non-Regular Languages
1. Union Operation : Set of Non-Regular languages is NOT Closed under Union Operation.
For counter example, Consider $L = \left \{ a^nb^n | n \geq 1 \right \}$ and $\overline{L}$...Both are Non-regular languages. But $L \cup \overline{L}$ = $\Sigma^*$ which is Regular language.
2. Intersection Operation : Set of Non-Regular languages is NOT Closed under Intersection Operation.
For counter example, Consider $L = \left \{ a^nb^n | n \geq 1 \right \}$ and $\overline{L}$...Both are Non-regular languages. But $L \cap \overline{L}$ = $\phi$ which is Regular language.
3. Complementation Operation : Set of Non-Regular languages is Closed under Complementation Operation.
i.e. Complement of a Non-regular language is always a Non-regular language.
We can prove it by Contradiction.
Let $L$ be any Non-regular language. Now, for contradiction purpose, Assume $\overline{L}$ be Regular.
Now, Since $\overline{L}$ is Regular, so, $\overline{\overline{L}} $ = $L$ will be Regular, which Contradicts our assumption that $\overline{L} $ is non-regular.
So, If $L$ is non-regular then $\overline{L}$ is necessarily non-regular.
We can say that $L$ is Regular if and only if $\overline{L} $ is Regular.
MUST Watch: Closure Properties of Non-Regular Languages